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You have the following:

A Microsoft 365 E5 tenant

An on-premises Active Directory domain

A hybrid Azure Active Directory (Azure AD) tenant

An Azure Active Directory Domain Services (Azure AD DS) managed domain

An Azure Virtual Desktop deployment

The Azure Virtual Desktop deployment contains personal desktops that are hybrid joined to the on-premises domain and enrolled in Microsoft Intune.

You need to configure the security settings for the Microsoft Edge browsers on the personal desktops.

Solution: You create and configure a Group Policy Object (GPO) in the on-premises domain.

Does this meet the goal?